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Croatica Chemica Acta, Vol.77 No.1-2 Svibanj 2004.

Izvorni znanstveni članak

On the Robustness of Low-frequency Laser Control Schemes for Proton Transfer in Thioacetylacetone

Iva Tatić ; Department of Chemistry, Faculty of Science, University of Zagreb, Marulićev trg 19, 10000 Zagreb, Croatia
Nađa Došlić ; Department of Physical Chemistry, Ruđer Bošković Institute, Bijenička 54, 10000 Zagreb, Croatia

Puni tekst: engleski, pdf (211 KB) str. 83-88 preuzimanja: 162* citiraj
APA 6th Edition
Tatić, I. i Došlić, N. (2004). On the Robustness of Low-frequency Laser Control Schemes for Proton Transfer in Thioacetylacetone. Croatica Chemica Acta, 77 (1-2), 83-88. Preuzeto s https://hrcak.srce.hr/102649
MLA 8th Edition
Tatić, Iva i Nađa Došlić. "On the Robustness of Low-frequency Laser Control Schemes for Proton Transfer in Thioacetylacetone." Croatica Chemica Acta, vol. 77, br. 1-2, 2004, str. 83-88. https://hrcak.srce.hr/102649. Citirano 18.09.2018.
Chicago 17th Edition
Tatić, Iva i Nađa Došlić. "On the Robustness of Low-frequency Laser Control Schemes for Proton Transfer in Thioacetylacetone." Croatica Chemica Acta 77, br. 1-2 (2004): 83-88. https://hrcak.srce.hr/102649
Harvard
Tatić, I., i Došlić, N. (2004). 'On the Robustness of Low-frequency Laser Control Schemes for Proton Transfer in Thioacetylacetone', Croatica Chemica Acta, 77(1-2), str. 83-88. Preuzeto s: https://hrcak.srce.hr/102649 (Datum pristupa: 18.09.2018.)
Vancouver
Tatić I, Došlić N. On the Robustness of Low-frequency Laser Control Schemes for Proton Transfer in Thioacetylacetone. Croatica Chemica Acta [Internet]. 31.05.2004. [pristupljeno 18.09.2018.];77(1-2):83-88. Dostupno na: https://hrcak.srce.hr/102649
IEEE
I. Tatić i N. Došlić, "On the Robustness of Low-frequency Laser Control Schemes for Proton Transfer in Thioacetylacetone", Croatica Chemica Acta, vol.77, br. 1-2, str. 83-88, svibanj 2004. [Online]. Dostupno na: https://hrcak.srce.hr/102649. [Citirano: 18.09.2018.]

Sažetak
The paper investigates quantum control of the proton transfer reaction in a two-dimensional model system using terahertz (THz) laser fields. The model potential, tailored to MP2 data for thioacetylacetone, comprises the proton transfer and the heavy atom coordinates. Two distinct mechanisms of proton transfer are investigated: the resonant versus the tunneling one. The efficiency of laser control in both cases is tested against the instability of pulse characteristics. The study shows that while the resonant scheme allows efficient control for a large range of field parameters, the tunneling scheme is very sensitive to the pulse characteristics, and therefore experimentally hardly realizable.

Ključne riječi
low-frequency laser; proton transfer; thioacetylacetone

Hrčak ID: 102649

URI
https://hrcak.srce.hr/102649

Posjeta: 238 *