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Hrvatski meteorološki časopis, Vol. 43 No. 43/1, 2008.

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SEASONAL VARIABILITY OF AEROSOL COMPOSITION IN SWITZERLAND: A MODELLING STUDY

Sebnem Andreani-Aksoyoglu ; Laboratory of Atmospheric Chemistry (LAC), Paul Scherrer Institute, Switzerland
Johannes Keller ; Laboratory of Atmospheric Chemistry (LAC), Paul Scherrer Institute, Switzerland
M. Rami Alfarra ; Laboratory of Atmospheric Chemistry (LAC), Paul Scherrer Institute, Switzerland
Jisca Sandradewi ; Laboratory of Atmospheric Chemistry (LAC), Paul Scherrer Institute, Switzerland
Andre S.H. Prevot ; Laboratory of Atmospheric Chemistry (LAC), Paul Scherrer Institute, Switzerland

Puni tekst: engleski pdf 658 Kb

str. 282-286

preuzimanja: 561

citiraj

Sažetak

In this study, we applied the MM5/CAMx model system over Switzerland for winter and summer periods in 2006. The
focus is on the formation and transport of aerosols and the contribution of various sources to the aerosol formation both in winter
and summer seasons. Our model system uses three nested domains with 27 km (Europe), 9 km (central Europe) and 3 km
(Switzerland) resolutions. The concentrations of aerosol components are calculated for particle sizes smaller than 2.5 μm. The
model’s capability to reproduce the aerosol concentrations is investigated by comparing the model results with the measurements
performed during the same periods. In general, the modelled concentrations of inorganic aerosols agree quite well with the AMS
measurements, whereas organic aerosols are underestimated. The chemical composition of aerosols in summer differs from that in
winter. Both measurements and model predictions indicate that organic aerosols and particulate nitrate are the major components of
the winter aerosol composition in Switzerland. In summer, organic aerosols dominate the aerosol composition and they are mostly
secondary organic aerosols formed from the biogenic precursors. Recent measurements suggest that wood-burning emissions might
contribute significantly to the aerosol concentrations, especially in winter. The lack of wood burning emissions in emission
inventory could cause partly the underestimation of organic aerosols. The secondary organic aerosol (SOA) formation will be soon
improved by using a new model version where oligomerization and SOA formation from isoprene and sesquiterpenes are
implemented.

Ključne riječi

aerosol modelling; CAMx; SOA; biogenic emissions

Hrčak ID:

64257

URI

https://hrcak.srce.hr/64257

Datum izdavanja:

12.12.2008.

Posjeta: 910 *