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A Localized Atomic Orbital Description of the Rotational Barrier in Ethane

Keith H. Aufderheide ; Oglethorpe University, 4484 Peachtree Road, NE Atlanta, Georgia 30319, U.S.A.


Puni tekst: engleski pdf 19.196 Kb

str. 811-831

preuzimanja: 198

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Sažetak

The rotational barrier in ethane is analyzed in terms of localized
atomic orbitals (LAOs). It is discerned that the barrier can be
ascribed to energies representative of vicinal interactions between
C-H bonds. It is found that exchange energies are of special
importance. Variations in the vicinal interaction energies can
ultimately be traced to chaTge flows into and out of various vicinal
LAO distributions upon rotation, and the impetus for these charge
flows is easily rationalized based on simple physical considerations.

Ključne riječi

Hrčak ID:

194057

URI

https://hrcak.srce.hr/194057

Datum izdavanja:

14.1.1985.

Posjeta: 591 *