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Structural properties of a-Si1-xCx:H by SAXS and IR spectroscopy

Davor Gracin ; "R. Bošković" Institute, POB 1016, Bijenička 54, 10000 Zagreb, Croatia
Pavo Dubček ; "R. Bošković" Institute, POB 1016, Bijenička 54, 10000 Zagreb, Croatia


Puni tekst: engleski pdf 203 Kb

str. 131-140

preuzimanja: 70

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Sažetak

The a-Si1-xCx:H thin films, with carbon concentrations up to x = 0.3 deposited by means of a DC magnetron sputtering source, using benzene vapour as the origin of carbon atoms, were analysed by small-angle X-ray scattering (SAXS) and IR spectroscopy. The incorporation of carbon atoms in a-Si:H results in the appearance of IR absorption related to the Si-C and C-H bonds and a slight decrease of absorption related to Si-H bonds. By increasing the carbon concentration, stretching frequency of Si-H bonds increases. This frequency, which is related to the described changes, is considered to be the consequence of an increasing void volume ratio and/or void volume per each Si-H oscillator. The SAXS data of pure a-Si:H indicate ``particles" with the giro radius RG = 1.27 nm, which increases with the carbon content up to RG = 2.05 nm. These ``particles" are attributed to the clusters of small voids with dimensions up to several silicon vacancies.

Ključne riječi

a-Si1-xCx:H thin films; different carbon concentrations; DC magnetron sputtering; small angle X-ray scattering (SAXS); IR spectroscopy; stretching frequency of Si-H bonds; clusters of small voids

Hrčak ID:

300966

URI

https://hrcak.srce.hr/300966

Datum izdavanja:

1.7.1999.

Podaci na drugim jezicima: hrvatski

Posjeta: 582 *